Hi Shane, my guess is that it's a permissions problem that's preventing MoI from writing to the moi.ini file. It's probably that your old user account has ownership of the directory and the files and you need to take ownership of those on your new machine.
Try something like this on both the Application Support/Moi folder and the files in the folder too: http://osxdaily.com/2013/04/23/change-file-ownership-mac-os-x/
- Michael
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